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This work proposes a methodology for designing high-strength precipitation-hardened high entropy alloys (HEAs) with an FCC matrix and L12 precipitates. High-throughput solidification calculations were conducted using the CALPHAD method, evaluating 11,235 alloys in the Cr-Co-Ni-Al-Ti system under specific boundary conditions. The acquired information was used to filter the alloys, focusing on alloys exhibiting an FCC+L12 phase field at 750 °C, a solidification interval narrower than 100 °C, and a solvus temperature under 1100 çC. The filtered alloys were analyzed to estimate their solid solution and precipitation hardening contributions to yield strength, with antiphase boundary energy (APB) assessed using two models. Three alloys were selected for testing the proposed strategy, including one with the highest yield stress and others for comparison. These alloys were produced, processed, and characterized using DSC, synchrotron XRD, SEM, and TEM. The results showed that the desired microstructure was achieved, with the alloys consisting of an FCC matrix and a high-volume fraction of L12 precipitates. Tensile tests at room temperature, 650 °C, 750 °C, and 850 °C demonstrated that the proposed model predicts well the yield strength trends, demonstrating the potential of the proposed approach for accelerating the discovery and development of novel HEAs with tailored properties.